Harleys can be nasty on brassicas/mustards and they go after tomatoes, corn, beans, and peas. Agree with Jason, and I might go a bit further depending on your situation:
If you are not planting brassicas, mustards, tomatoes, corn, beans, and peas near the problem area then let them flower. You created a super trap crop. You are also looking for parasitic wasps and flies to come in and control the future generations this season. I would also plant other small-flowered plants to ensure the beneficials come in strong (like Jason always says).
If you are planting new brassicas/mustards, tomatoes, corn, beans, and peas anywhere near the existing ones:
- Hand-remove all adult/Nymph Harlequins (not much can predate them due to semi-hard/hard shells)
- Hand-remove all eggs you find, regardless of type (no time for fast beneficials)
- Remove all brassicas material, mulch, and weeds that are in the block or small bed (if it is manageable)
- Plant your new plants and cover with floating row covers (like agribon or reemay)
- Grow your brassicas under the cloth most/all of the season this year (Harleys tend to make 2 generations or more a year)
- Plant small-flowered plants on the borders or inter-planted and don't monocrop if you can avoid it
- Keep your brassica beds weed-free since Harleys live in and around them as well
If the Harleys come back hard again, the following can be used, but they can kill beneficials as well, so only apply to known problem plants:
- Garlic spray with some added dish soap (homemade or bought) <-- I use this outdoors
- Insecticidal Soap (homemade or bought) <-- I use indoors
- Canola or Veg Oil-based Horticulural Oil (sometimes called Dormant, Summer or Superior Oil) <-- I use this when bees are not around
- Kaolin Clay Spray (sold as a powder then mixed with water) <-- I have never used this but some friends like it
You can find the above sprays at many garden stores and can be OMRI-compliant if you go down that path. If you are looking for a more dark-side

approach, look into Petroleum-based Dormant/Superior Oils, Pyrethins, Rotenone, Spinosad, Neem Oil, Beauveria Bassiana, and a complete last-resort Sabadilla powders (this stuff is downright terrible) but nuclear option. Most of these can kill the good guys including bees.